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This book shows the electronic, optical and lattice-vibration properties of the two-dimensional materials which are revealed by the Raman spectroscopy. It consists of eleven chapters covering various Raman spectroscopy techniques (ultralow-frequency, resonant Raman spectroscopy, Raman imaging), different kinds of two-dimensional materials (in-plane isotropy and anisotropy materials, van der Waals heterostructures) and their physical properties (double-resonant theory, surface and interface effect). The topics include the theory origin, experimental phenomenon and advanced techniques in this area. This book is interesting and useful to a wide readership in various fields of condensed matter physics, materials science and engineering.